Fagkonferansen i Budapest omhandler fremlegg av forskningsresultater innenfor overflate- og kolloidkjemiske problemstillinger inkludert en del nanoteknologi. Konferansen ble avholdt fra og med mandag 18.09 til og med fredag 22.09. Hver dag består av to plenarforedrag og en rekke kortere innlegg med to parallelle sesjoner. I tillegg kommer plakatforedragene som avholdes på ettermiddag og kveldstid. Vi hadde et plakatforedrag første dagen. Konferansen hadde 425 påmeldte deltakere. Nedenfor er sammendraget fra vårt bidrag presentert. Dette er nødvendigvis skrevet på Engelsk:

 

Adsorption of phenol and benzyl alcohol onto surfactant modified silica.

 

Geir Martin Førland* and Anne Marit Blokhus**

 

* Institute for Aquaqulture- Chemistry- and Biochemistry subjects, Faculty of Engineering, Bergen University College, P.O.Box 7030, N-5020 Bergen, Norway

**Department of Chemistry, University of Bergen, Allégt. 41, N-5007 Bergen, Norway

 

 

The formation of micelles is aided by a cooperative interaction due to van der Waals forces between the hydrocarbon chains of the surfactant molecules. The same interaction is believed to be responsible for the formation of surfactant aggregates on solid surfaces. Previous data has shown a broad variation in the structure of these adsorbed aggregates depending on the system studied (1-3). However, the interior of the aggregates is extremely similar to those of a micelle. This gives an excellent situation for incorporation of hydrophobic components just as ordinary micelles are known to do.

 

Here, the adsorption of the surfactant, dodecyltrimethylammonium bromide (DTAB) and the co-adsorption of the additives, phenol and benzyl alcohol, onto silica is investigated. With a constant DTAB concentration and varying alcohol concentration the results show an increasing adsorption of alcohol with increasing alcohol concentration. In the solution containing a phenol concentration of 0.29 M, the mole-ratio of alcohol to surfactant at the solid surface reaches approximately 4.3. The corresponding mole-ratio for the solution containing 0.25 M benzyl alcohol is 6.6. This indicates that the surfactant aggregates at the silica surface has a very high ability to incorporate phenol and benzyl alcohol.

 

The adsorption density of DTAB onto silica is found to increase at low phenol and benzyl alcohol concentrations before a maximum in the adsorption is reached at an alcohol concentrations of about 0.05M. At the maximum surfactant adsorption density, the mole-ratio of alcohol to surfactant on the silica surface is approximately 1.0. A further increase in the concentration of the alcohols gives a readily decrease in the adsorption data of the DTAB while the adsorption of alcohol continues to increase. However, the slope of the line, when plotting the alcohol a  adsorption capacity against the alcohol concentration, decreases as the alcohol concentration increases. The result indicates that the surfactant aggregates increases and becomes large mixed surfactant-alcohol aggregates when alcohol is added in the low concentration range. In the higher concentration range, where the alcohol continues to adsorb while the surfactant starts to desorb, the mixed aggregates seem to contain several alcohol molecules for each surfactant molecule.

References

  1. J-F. Liu, W.A. Ducker, J. Phys. Chem. B 1999, 103:8558.
  2. L. Kovacs, G.G. Warr, Langmuir, 2002, 18:4790
  3. G.G. Warr, Current Opinion in Colloid & Interface Science, 2000, 5:88